Published in Nature Physics 16, 526 (2020).

Proximity-induced superconducting gap in the quantum spin Hall edge state of monolayer WTe2

Felix Lüpke1, Dacen Waters1, Sergio C. de la Barrera1, Michael Widom1, David G. Mandrus2,3,4, Jiaqiang Yan2, Randall M. Feenstra1, and Benjamin M. Hunt11
1Dept. Physics, Carnegie Mellon University, Pittsburgh, PA 15213, USA
2Materials Science and Technology Division, Oak Ridge National Laboratory, Oak Ridge, TN 37831, USA
3Department of Materials Science and Engineering, University of Tennessee, Knoxville, TN 37996, USA
4Department of Physics and Astronomy, University of Tennessee, Knoxville, TN 37996, USA

Abstract

The quantum spin Hall (QSH) state was recently demonstrated in monolayers of the transition metal dichalcogenide 1T’-WTe2 and is characterized by a band gap in the two-dimensional (2D) interior and helical one-dimensional (1D) edge states [1–3]. Inducing superconductivity in the helical edge states would result in a 1D topological superconductor, a highly sought-after state of matter [4]. In the present study, we use a novel dry-transfer flip technique to place atomically-thin layers of WTe2 on a van der Waals superconductor, NbSe2. Using scanning tunneling microscopy and spectroscopy (STM/STS), we demonstrate atomically clean surfaces and interfaces and the presence of a proximity-induced superconducting gap in the WTe2 for thicknesses from a monolayer up to 7 crystalline layers. At the edge of the WTe2 monolayer, we show that the superconducting gap coexists with the characteristic spectroscopic signature of the QSH edge state. Taken together, these observations provide conclusive evidence for proximity-induced superconductivity in the QSH edge state in WTe2, a crucial step towards realizing 1D topological superconductivity in this van der Waals material platform.

Click here for preprint of paper, in pdf format.

Return to Home Page of Feenstra group